Improved Simulations of Global Black Carbon Distributions by Modifying Wet Scavenging Processes in Convective and Mixed?Phase Clouds

نویسندگان

چکیده

In-cloud wet scavenging dominates the removal of aerosols in atmosphere, but is not well represented climate models. Aircraft measurements black carbon (BC) concentrations suggest that models commonly overestimate BC upper troposphere tropics by more than one order magnitude underestimate burdens polar latitudes. In this study, we improved in-cloud parameterizations for convective clouds and mixed-phase to better characterize abundances remote atmosphere (remote oceans regions) with a global model, CAM5-ATRAS2. The modified processes model achieved realistic simulation over both Arctic. new, unified scheme vertical transport during deep convection generally reproduced observed low mixing ratios (about 0.1 ng kg?1) middle tropics, Wegener–Bergeron–Findeisen process (WBF) lowered efficiency from consequently increased Arctic about factor 2. direct radiative forcings 20% globally (from 0.26 0.31 W m?2), importantly 2 0.09 0.18 m?2). Our results indicated good agreement between modeled could be obtained without requiring relatively short lifetime (?4 days) suggested previous studies.

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ژورنال

عنوان ژورنال: Journal Of Geophysical Research: Atmospheres

سال: 2021

ISSN: ['2169-8996', '2169-897X']

DOI: https://doi.org/10.1029/2020jd033890